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Another notable inmate was Jonathan Pollard, a former U.S. Navy analyst who was convicted of spying for Israel. His case remains controversial, given the lasting national security implications. John Hinckley Jr., known for attempting to assassinate President Ronald Reagan, also resided in FCI Butner, where his mental health needs were a primary focus. This highlighted the complex's role in providing psychiatric care within the penal system.
Additionally, figures such as Frank Calabrese Sr., notorious for his connection to organized crime, further diversified the inmate population at FCI Butner. With a mix of high-profile criminals, the facility has garnered attention in popular culture, even appearing in fictional works like Better Call Saul.