The interrogation of Morpheus. Iconic scene from an iconic movie.
I'm not sure if it's intentional or not but from the street below you can actually see the light inside the window flicker. Like the spark of an idea in the mind of Morpheus.
Using the window as the center of his head is certainly intentional.
The window definitely is. But the light inside is a bit dodgy and is flickering, I don't think that part was intentional but it kinda makes it even better.